Process intensification of hydrogen production by steam reforming of methane over structured channel packing catalysts

نویسندگان

چکیده

The industrial methane steam reforming reaction usually employs particulate catalyst that are easy to prepare and cost-effective, but suffer from problems such as high reactor pressure drop low overall utilization. In this study, the Ni-Al 2 CaO 4 powder prepared by equal volume impregnation method was subjected particle size control using a pressing method, made into particles of different sizes. Some catalysts were filled honeycomb structures with cordierite metal substrates, respectively, regular channel packing catalysts. differences in conversion rate, H /CO selectivity, among three compared, influence on performance systematically explored. results showed under same conditions, increased, rate increased. two substrates similar levels, substrate exhibited higher due its excellent thermal conductivity. Compared single-particle size, reduced more than 25%. Under conditions gas hourly space velocity 2000 h -1 , temperature 700 °C, water-to-carbon ratio 3, 40-60 mesh 7% increase reaching 95.2%.

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ژورنال

عنوان ژورنال: E3S web of conferences

سال: 2023

ISSN: ['2555-0403', '2267-1242']

DOI: https://doi.org/10.1051/e3sconf/202338502018